Crystal structure and luminescence properties of a new nanostructure lead(II) complex: a precursor for preparation of pure phase nanosized PbO

Document Type: Research Article

Authors

1 Department of Chemistry, Payame Noor University, PO Box 19395-3697 Tehran, Iran

2 Department of Chemistry, Miyandoab Branch, Islamic Azad University, Miyandoab, Iran

Abstract

The reaction of 1,3-diphenylpropane-1,3-dione (HL) ligand with lead(II) nitrate under hydrothermal conditions led to the formation of a novel lead complex with singular structural features. The characterization of title complex was performed by spectroscopy methods such as 1H NMR, UV, and IR and elemental analyses (CHN) and crystal structure of prepared lead (II) complex was determined by single-crystal X-ray diffraction. The facile and productive sonochemical method was used to prepare nano-size particles of the title complex at room temperature. The prepared nano-size-complex was characterized by elemental analysis, scanning electron microscopy (SEM), IR spectroscopy and X-ray powder diffraction (XRD). The nano-size lead oxides that prepared by calcination of the nano-size complex and crystalline bulk complex showed the initial particle size of the precursor is influential on the particle size of the derived PbO nanoparticles. Optical property investigation of the PbO nanoparticles at room temperature showed that the size of PbO nanoparticles has an important role on their optical behavior.

Graphical Abstract

Crystal structure and luminescence properties of a new nanostructure lead(II) complex: a precursor for preparation of pure phase nanosized PbO

Keywords


[1]     L. Aboutorabi,; A. Morsali,; Structural transformations and solid-state reactivity involving nano lead(II) coordination polymers via thermal, mechanochemical and photochemical approaches. Coord. Chem. 310 (2016) 116-130.
[2]     A.A. Abd-Rabou,; H.H. Ahmed, CS-PEG decorated PLGA nano-prototype for delivery of bioactive compounds: A novel approach for induction of apoptosis in HepG2 cell line. Adv. Med. Sci. 62 (2017) 357-367.
[3]     T. Alizadeh,; S.A. Naser, Chiral resolution of salbutamol in plasma sample by a new chiral ligand-exchange chromatography method after its extraction with nano-sized imprinted polymer. J. Chromatogr. B. (2016) 1009–1010, 96-106.
[4]     A.A. Bazrafshan, M. Ghaedi, Z. Rafiee, S. Hajati, A. Ostovan, Nano-sized molecularly imprinted polymer for selective ultrasound-assisted microextraction of pesticide Carbaryl from water samples: Spectrophotometric determination. J. Colloid. Interface. Sci. 498 (2017) 498, 313-322.
[5]     M. Bayat; S. Kamali, Computational landscape of the formation and nature of bond in the “1 + 1” versus “1 + 2” nano-sized complexes of some adducts of N-heterocyclic carbenes (NHC) with heavy elements of group II (Ca, Sr, Ba) metallocenes. J. Mol. Liq. 222 (2016) 953-962.
[6]     X. Chen, S. Chen; P.M. Clequin, W.T. Shoulders; Gaume, R. Combustion synthesis of lead oxide nanopowders for the preparation of PMN–PT transparent ceramics. Ceram. Int. 41 (2015) 755-760.
[7]     R. Ding; X. Li; W. Shi; Q. Xu; E. Liu, One-pot solvothermal synthesis of ternary Ni-Co-P micro/nano-structured materials for high performance aqueous asymmetric supercapacitors. Chem. Eng. J. 320 (2017) 376-388.
[8]     A.F. Esfanjani; S.M. Jafari, Biopolymer nano-particles and natural nano-carriers for nano-encapsulation of phenolic compounds. Colloids. Surf. B. 146 (2016) 532-543.
[9]     Z. Fereshteh; M. Salavati-Niasari; Effect of ligand on particle size and morphology of nanostructures synthesized by thermal decomposition of coordination compounds. Adv. Colloid. Interface. Sci. 243 (2017) 86-104.
[10] H. Ghasempour; T.A. Azhdari; A. Morsali, Ultrasonic-assisted synthesis and structural characterization of two new nano-structured Hg(II) coordination polymers. Ultrason. Sonochem. 27 (2015) 503-508.
[11] L. Guan; Y.A. Wang, novel second-order non-linear optical coordination polymer with three-fold interpenetrated CdSO4-type network constructed by carboxylate–sulfonate ligands and strontium ions. J. Solid. State. Chem. 230 (2015) 243-248.
[12] E. He; S. Wang; Y. Li; Q. Wang, Enhanced tribological properties of polymer composites by incorporation of nano-SiO2 particles: A molecular dynamics simulation study Computational. Mater. Sci. 134 (2017) 93-99.
[13] H.J. Im; S.W. Lee, Two-dimensional 3d–4f coordination polymers based on compartment compounds: [NiLn(L)(NO3)2(4-pca)(H2O)] (Ln = Nd, Eu, Tb; H2L = 1,3-bis((3-methoxysalicylidene)amino)propane); 4-Hpca = pyridine-4-carboxylic acid). Polyhedron. 110 (2016) 24-30.
[14] R. Kruszynski, Commenting the “Sonochemical synthesis of two new zinc(II) 1,10-phenanthroline coordination supramolecular compounds: New precursors to produce nano-sized zinc(II) oxide”. Ultrason. Sonochem. 39 (2017) 218.
[15] V.V. Krisyuk; I.A. Baidina; A.E. Turgambaeva; S.U. kyzy; I.V. Korolkov; T.P. Koretskaya; I.K. Igumenov, Structure and thermal properties of Pb(II) complex with functionalized β-diketonate. J. Organomet. Chem. 819 (2016) 115-119.
[16] J.H. Lee; S.Y. Im; S.W. Lee, 1D and 2D Zn–Ln coordination polymers based on compartment compounds: [ZnLn(L)(NO3)2(4-ppa)(EtOH)] and [ZnLn(L)(NO3)2(4-pca)(H2O)] (Ln = Eu, Tb; H2 L = 1,3-bis((3-methoxysalicylidene)amino)propane; 4-Hppa = 4-pyridinepropionic acid; 4-Hpca = 4-pyridinecarboxylic acid). Polyhedron. 118 (2016) 125-132.
[17] R. Li; F. Xiao; S. Amirkhanian; Z. You; J. Huang, Developments of nano materials and technologies on asphalt materials – A review. Constr. Build. Mater. 143 (2017) 633-648.
[18] J.G. Małecki; A. Maroń, Luminescence properties of copper(I), zinc(II) and cadmium(II) coordination compounds with picoline ligands. J. Lumin. 186 (2017) 127-134.
[19] G. Mills; Z. Li; D. Meisel, Photochemistry and spectroscopy of colloidal arsenic sesquisulfide. J.  Phys. Chem. 92 (1988) 822-828.
[20] J. Ngoune; J.J. Anguile; J. Nenwa; G. Djimassinga; C. Pettinari; E. Álvarez; L. Pandolfo, Synthesis, characterization and molecular structure of a zinc(II) formate-2,2′-bipyridine mono-dimensional coordination polymer. Comparison with other 2,2-bipyridine coordination compounds. Inorg. Chim. Acta. 453 (2016) 263-267.
[21] S. Naveenraj; G.J. Lee; S. Anandan; J.J. Wu, Nanosized tantala based materials – synthesis and applications. Mater. Res. Bull. 67 (2015) 20-46.
[22] D.D. Perrin; W.L. Armaredo; D.R. Perrin, Purification of Laboratory Chemicals, 2nd Ed. Pergamon Press, Oxford, 1980.
[23] S. Rostamnia; A. Morsali, Size-controlled crystalline basic nanoporous coordination polymers of Zn4O(H2N-TA)3: Catalytically study of IRMOF-3 as a suitable and green catalyst for selective synthesis of tetrahydro-chromenes. Inorg. Chim. Acta. 411 (2014) 113-118.
[24] S.S. Sreejith; N. Mohan; N. Aiswarya; M.R. Prathapachandra Kurup, Inclusion, pseudo-inclusion compounds and coordination polymer of Pd(II), Zn(II) and Cd(II) from salen-type Schiff base ligand with a 1,3-diimino spacer group: Crystal structures, spectroscopic and thermal studies. Polyhedron. 115 (2016) 180 -192.
[25] M.J. Soltanian Fard; P. Hayati; A. Firoozadeh; J. Janczak; Sonochemical synthesis of two new zinc(II) 1,10-phenanthroline coordination supramolecular compounds: New precursors to produce nano-sized zinc(II) oxide. Ultrason. Sonochem. 37 (2017) 286-297.
[26] S. Suckert; H. Terraschke; H. Reinsch; C. Näther, Synthesis, crystal structures, thermal, magnetic and luminescence properties of Mn(II) and Cd(II) thiocyanate coordination compounds with 4-(Boc-amino)pyridine as co-ligand. Inorg. Chim. Acta. 461 (2017) 290-297.
[27] A.V. Savchenkov; M.S. Grigoriev, P.A. Udivankin; D.V. Pushkin, L.B. Serezhkina, Maleate ions as ligands in crystal structures of coordination compounds, including two uranyl complexes. Polyhedron. 127 (2017) 331-336.
[28] M. Sumesh; U.J. Alengaram, M.Z. Jumaat, K.H. Mo, M.F. Alnahhal, Incorporation of nano-materials in cement composite and geopolymer based paste and mortar –A review. Constr. Build. Mater. 148 (2017) 62-84.
[29] P.B. Taunk, R. Das, D.P. Bisen, R.K. Tamrakar, Synthesis and characterization of pure and Zn doped lead hydroxide nano structure through chemical root method. Optik.  Int.  J.  Light. Electron.  Opt.127 (2016) 4995-5012. 
[30] Q. Zhou, J. Qian, C. Zhang, Three interesting coordination compounds based on metalloligand and alkaline-earth ions: Syntheses, structures, thermal behaviors and magnetic property. J. Mol. Struct. 1119 (2016) 340-345.
[31] K.F. Zare, V. Safarifard, K.S. Karbalaei, A. Morsali, Ultrasound-assisted synthesis of nano-structured 3D zinc(II) metal–organic polymer: Precursor for the fabrication of ZnO nano-structure. Ultrason. Sonochem. 23 (2015) 238-245.
[32] L. Zhou, X. Zhang, Y. Chen, Facile synthesis of Al-fumarate metal–organic framework nano-flakes and their highly selective adsorption of volatile organic compounds. Mater. Lett. 197 (2017) 224-227.
[34] L. Zhang, Y. Zhou, G. Shi, X. Sang, C. Ni, Preparations of hyperbranched polymer nano micelles and the pH/redox controlled drug release behaviors. Mater. Sci. Eng. C. 79 (2017) 116-122.
[35] H. Zhou, M. Su, P.H. Lee, K. Shih, Synthesis of submicron lead oxide particles from the simulated spent lead paste for battery anodes. J.  Alloys. Compd. 690 (2017) 101-107.